I just took a look at graysky's guide. Seems overly long and complicated because he tried to cover everything in one post instead of breaking things down into separate topics.
I use primarily Gigabyte motherboards so, yet again, the BIOS is different. Second, even with one manufacturer's line, less expensive motherboards will not have all the settings that the more expensive models have.
Memory clock dividers are one of those things that everybody handles differently.
Here's my advice (yes, more guides):
This should be your first stop.
HOWTO: Overclock C2Q (Quads) and C2D (Duals) - Guide v1.6.1
http://www.tomshardware.com/forum/240001-29-howto-overc...
Next stop should be a guide for your particular motherboard. Google is your friend.
Go through the guides. Then take your core voltage off Auto and set your memory voltage to factory recommended values. Change the System Memory Multiplier (or whatever your BIOS calls it - Asus uses "straps" for their Intel chipsets) from AUTO to 2.00, 2.00B, or 2.00D - whichever you need to set the Memory Frequency to twice the FSB. Then when you increase the FSB, the memory clock will rise in in proportion with it. At an FSB of 266 MHz, your memory clock should be at 533 MHz.
Download CPU-Z to check your FSB:RAM ratio. It should be a 1:1 ratio.
Warning - confusion factor between what the BIOS calls things and what CPUZ calls things. What the BIOS calls "memory frequency" is actually the memory clock. What CPUZ calls "memory frequency" is half the memory clock - DDR2 RAM, remember? It transfers two chunks of data each bus cycle. What you want in CPUZ is a 1:1 FSB:RAM ratio. With a 333 MHz FSB frequency, your RAM clock should be 667 MHz.
Overclocking memory doesn't accomplish much - especially in a Core2 system - besides limiting your CPU overclock where the real speed comes from. Here's one place where we discuss that:
http://www.tomshardware.com/forum/251715-29-ratio-myth
You have another problem. The G33 is an "economy" chipset. That means two things. First, you are not going to have all the usual overclocking options (including the sync setting that you cannot find), hence the advice to look for a guide for your specific motherboard. And second, I doubt if you are going to be able to push the FSB frequency much past 333 MHz. That means that the capabilities of your DDR2-1000 memory are going to be largely wasted.
Don't exceed 1.5 volts on the CPU cores and using CoreTemp or RealTemp, keep your core temps under 70 C.
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Overclocking since 1978 - Z80 (TRS-80) from 1.77 MHz to 2.01 MHz