You have to go with another of what you have. You could pair it with a 5850 or 5870 but they scale down to match your 5830 so you would be paying extra money for no added performance. There is a chart on the AMD website that you can go and have a look at it shows what goes with what.
EVERYTHING... lol no, 5830 is most logical what you should get for CF if you have a 5830, you can only match 5830 to 5850, 5830 and 5870, but they will be limited to 5830's performance levels